Photos app allows you to remove and rearrange photos in an album. To open an album, just double-click it. If you want to order photos by date, then choose "View" and select "Keep Sorted By Date" option. If you want to rearrange photos manually, then drag the photos into the order that you want. Photos app allows you to select a key photo for an album. It represents the album in the Photos window. To do so, Double-click an album to open it and select the photo which you want as the key photo. Choose "Image" and then select "Make Key Photo" option.
To remove photos from an album, select the photos and click "Delete" or choose "Image" and then click "Remove Photos from Album" option. The photos are removed from this specific album. By mistake you remove a photo from an album, then chose "Edit" and then select "Undo" to restore it.
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