You can remove files that you don't want to store in iCloud Drive by using the iClloud Drive app on iCloud.com. When you remove files, you can reduce the amount of iCloud storage space which you are using. If you remove a file from iCloud Drive on iCloud.com, then it is also removed from all your devices which set up to use iCloud Drive. To remove files from iCloud Drive, go to iCloud Drive on iCloud.com i.e. https://www.icloud.com/#iclouddrive. Select the files which you want to remove and click "Trash" button located in the iCloud Drive toolbar. If you do not see iCloud Drive on iCloud.com, then your account just has access to iCloud web-only. You can access to other iCloud features by setting up iCloud on your Mac or iOS device.
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